Whilst I don't think the mountain itself is particularly attractive, I do think that a visit to Pachnes - the highest point in the Lefka Ori or White Mountains on Crete - is a beautiful destination. For me the memories of a 2-day solo trip there using public transport from Chania to Omalos will last much longer than those of climbing Psiloritis or Dikti.
I also think that Gingilos is a beautiful Cretan mountain, in an absolutely stunning location. Climbing it is well worth it for the extensive views it gives over the White Mountains, with the Samarian Gorge between.
Now, had you asked about a beautiful bivouac site in Greece, I'd then be recommending Katsivelli as an absolutely superb location, just within stiking distance of Pachnes. What a place to stay - so isolated and so peaceful. I hope to finish preparing a trip report on this in the near future.